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This question is about jobs.
You need to get a working visa from the British Embassy in the United States in order to get a job in London as an American.
In addition, obtaining a work visa is a process that can only be initiated by a British company or employer who wants to hire you and is able to demonstrate why you (an American) fit the job listing better than any candidate from the UK and the European Union.
So, the first step is to reach out to employers in London and try to find positions that you are uniquely qualified for. If the employer finds this to be the case, they will start the process of getting you a work visa.

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